Impact of higher-order exchange on the lifetime of skyrmions and antiskyrmions

dc.contributorUniversity of Icelanden
dc.contributorHáskóli Íslandsis
dc.contributor.authorSchrautzer, Hendrik
dc.contributor.authorGoerzen, Moritz A.
dc.contributor.authorBeyer, Bjarne
dc.contributor.authorHaldar, Soumyajyoti
dc.contributor.authorBessarab, Pavel F.
dc.contributor.authorHeinze, Stefan
dc.contributor.departmentFaculty of Physical Sciences (UI)en
dc.contributor.departmentRaunvísindadeild (HÍ)is
dc.contributor.schoolSchool of Engineering and Natural Sciences (UI)en
dc.contributor.schoolVerkfræði- og náttúruvísindasvið (HÍ)is
dc.date.accessioned2026-11-10T12:41:03Z
dc.date.available2026-11-10T12:41:03Z
dc.date.issued2026-03-23
dc.descriptionVersion of record. Published in npj Computational Materials 12, 123 (2026), https://doi.org/10.1038/s41524-026-02034-9. Received 7 November 2025, accepted 2 March 2026. License of this item: CC BY 4.0.en
dc.description.abstractReliable control of skyrmion lifetime is essential for realizing spintronic devices, yet the role of higherorder exchange—which can lead to skyrmion stabilization—remains largely unexplored. Here we calculate lifetimes of isolated skyrmions and antiskyrmions at transition-metal interfaces based on an atomistic spin model that includes all fourth-order exchange terms. Within harmonic transition-state theory, we evaluate both energetic and entropic contributions and find substantially enhanced lifetimes when higher-order exchange is included. The four-spin four-site interaction raises the energy barrier and lowers the curvature of the energy landscape at the collapse saddle point, increasing the pre-exponential factor. We show that skyrmions and antiskyrmions can remain thermally stable even without Dzyaloshinskii-Moriya interaction (DMI), and that tuning the four-spin term by a small amount modulates the prefactor over orders of magnitude. Our results identify higher-order exchange as a promising route to stabilize topological magnetic textures—in particular in systems lacking DMI—and to engineer their thermally activated decay.en
dc.description.sponsorshipIcelandic Research Fund, grant no. 239435 Icelandic Research Fund, grant no. 2410333 Icelandic Research Fund, grant no. 217750 University of Iceland Research Fund, grant no. 15673 Swedish Research Council, grant no. 2020-05110 Crafoord Foundation, grant no. 20231063 Deutsche Forschungsgemeinschaft (DFG), SPP2137 "Skyrmionics", project no. 462602351 Deutsche Forschungsgemeinschaft (DFG), project no. 418425860en
dc.description.versionPeer Reviewed
dc.format.extent123; 1-14.
dc.identifier.citationSchrautzer, Hendrik, Goerzen, Moritz A., Beyer, Bjarne, Haldar, Soumyajyoti, Bessarab, Pavel F. & Heinze, Stefan. (2026). Impact of higher-order exchange on the lifetime of skyrmions and antiskyrmions. Springer Nature, npj Computational Materials 12, 123; 1-14.
dc.identifier.doihttps://doi.org/10.1038/s41524-026-02034-9
dc.identifier.journalnpj Computational Materials
dc.identifier.urihttps://hdl.handle.net/20.500.11815/9051
dc.language.isoen
dc.publisherSpringer Natureen
dc.relation.ispartofseries12
dc.relation.urlhttps://www.nature.com/articles/s41524-026-02034-9
dc.rightsinfo:eu-repo/semantics/openAccess
dc.subjectMagnetismen
dc.subjectMagnetic skyrmionsen
dc.subjectAntiskyrmionsen
dc.subjectHigher-order exchange interactionsen
dc.subjectHarmonic transition state theoryen
dc.subjectSkyrmion lifetimeen
dc.subjectAtomistic spin simulationsen
dc.subjectSegulmagnis
dc.subjectEðlisfræðiis
dc.subjectStærðfræðiis
dc.subjectSegulstraumfræðiis
dc.titleImpact of higher-order exchange on the lifetime of skyrmions and antiskyrmionsen
dc.typeinfo:eu-repo/semantics/article
dcterms.licensePublished under the Creative Commons Attribution 4.0 International License (CC BY 4.0), https://creativecommons.org/licenses/by/4.0/. © The Author(s) 2026.

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